After the Territorial Army began to expand following a Government announcement in March 1939, the Liverpool Scottish formed a second battalion. Mobilisation was later authorised, but both battalions would remain in Britain for the duration of the Second World War. The 2nd Battalion converted to artillery in 1942 as the 89th Anti-Tank Regiment, Royal Artillery. In addition, the Liverpool Scottish supplied drafts to other units, principally to the Cameron Highlanders, and formed contingents for the embryonic "Independent Companies" that became the Army "Commandos".
The Liverpool Scottish contributed a troop to the composite No. 4 Independent Company, which also contained troops from the King's Regiment and South Lancashires, collectively under the command of Major J.R. Paterson — an officer from the Scottish. Formed on 21 April 1940, at Sizewell, the company soon after embarked aboard the Ulster Prince, bound for Norway to join the Allied campaign against Germany. After landing in early May, No. 4 Company relieved a French force and occupied positions near Mosjoen. The company, in conjunction with others, operated under the aegis of Scisserforce, commanded by Brigadier Colin Gubbins. When a German landing cut off Mosjoen from the north on 11 May, No. 4 Company had to be evacuated by a Norwegian steamer and transported to Sandnessjøen, then to Bodø with No. 5 Company.
By the 24th, Allied troops had established a line of defence near the town of Pothus to facilitate the defence of Bodø against Germany's northern advance. While his forces were engaged in battle, Brigadier Gubbins was informed that the British Government had decided to evacuate northern Norway. The withdrawal of Allied forces commenced on 29 May, with Nos. 1 and 4 Companies being embarked on two destroyers carrying other passengers, including administrative personnel and wounded.
After returning to Britain, the Liverpool Scottish troop obtained approval from the Government to readopt the kilt as an integral part of its Battle Dress. The Commando units and the independent companies consolidated later in the year into "Special Service" battalions, administered by a single brigade. For various reason, the system proved unpopular and in 1941 the battalions were sub-divided, reverting to distinct Commando units. The 1st Special Service Battalion, which had absorbed No. 4 Company, became Nos. 1 and 2 Commando - the later including a number of the Liverpool Scottish, designated as 5 Troop.
In March 1942, the troop participated with 2 Commando in the raid on St Nazaire, codenamed Operation Chariot. Conceived to neutralise the western French port as an Atlantic sanctuary for the battleship Tirpitz,[Operation Chariot involved 611 men, the antiquated lend-lease destroyer Campbeltown, and numerous small craft. The Campbeltown was converted into a platform designed to deliver 9,600 pounds (4,400 kg) of explosives, and her appearance was reconfigured to resemble a German destroyer.
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